Measurements of kinetic processes in a self-sustained discharge XeF laser

Measurements are presented for processes occurring in XeF self-sustained discharges including fluorescence, gain, and absorption at different wavelengths as a function of F2, Xe, and He partial pressures. Time-correlated oscillograms are given for the laser discharge current, metastable XeF small-signal gain at 351.1 nm, transient absorptions at 333.6 and 363.8 nm, metastable-XeF B-state sidelight emission at about 350 nm, metastable-F emission at 634.8 nm, and metastable-F emission at 731.1 nm. It is found that He atoms are necessary for the production of metastable-XeF in its lower vibrational levels and that radiative processes and He quenching are the primary mechanisms for metastable-XeF decay. For small-signal gains of as low as about 8%/cm, the transient absorption at the laser wavelength may be as large as about 1-2%/cm.