The influence of dynamics on two-dimensional model results - Simulations of C-14 and stratospheric aircraft NO(x) injections

The influence of dynamics on model results is investigated via a 2D photochemical model. Three representations of atmospheric transport are tested in order to simulate total ozone and C-14 amounts after nuclear tests in the early 1960s. Three scenarios of NO(x) injections from a proposed fleet of stratospheric aircraft and their effects on ozone are simulated. The three dynamical formulations used are Dynamics A, a base dynamics used in previous work with this model; Dynamics B, a strong circulation dynamics discussed by Jackman et al. (1989); and Dynamics C, the dynamics used by Shia et al. (1989). The advective component of the stratosphere to the troposphere mass exchange rate is largest for Dynamics B (5.8 x 10 exp 17 kg/yr) and smallest for Dynamics C (1.4 x 10 exp 17 kg/yr), with the advective strat/trop exchange rate for Dynamics A (2.4 x 10 exp 17 kg/yr) being these two extremes. Ozone depletion from NO(x) injections of stratospheric aircraft showed a strong sensitivity to dynamics.