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Extreme Ozone Loss Following Nuclear War Results in Enhanced Surface Ultraviolet Radiation For the first time, we use a modern climate model with interactive chemistry including the effects of aerosols on photolysis rates to simulate the consequences of regional and global scale nuclear wars (injecting 5 and 150 Tg of soot respectively) for the ozone layer and surface ultraviolet (UV) light. For a global nuclear war, heating in the stratosphere, reduced photolysis, and an increase in catalytic loss from the Hox cycle cause a 15 year-long reduction in the ozone column, with a peak loss of 75% globally and 65% in the tropics. This is larger than predictions from the 1980s, which assumed large injections of nitrogen oxides (NOx),but did not include the effects of smoke. NOx from the fireball and the fires provide a small (5%) Increase to the global average ozone loss for the first few years. Initially, soot would shield the surface from UV-B, but UV Index values would become extreme: greater than 35in the tropics for 4years, and greater than 45during the summer in the southern polar regions for 3 years. For a regional war, global column ozone would be reduced by 25% with recovery taking 12 years. This is similar to previous simulations, but with a faster recovery time due to a shorter lifetime for soot in our simulations. In-line photolysis provides process specific action spectra enabling future integration with biogeochemistry models and allows output that quantifies the potential health impacts from changes in surface UV for this and other larger aerosol injections.
Document ID
20210021315
Acquisition Source
Goddard Space Flight Center
Document Type
Accepted Manuscript (Version with final changes)
Authors
Charles G. Bardeen ORCID
(National Center for Atmospheric Research Boulder, Colorado, United States)
Douglas E. Kinnison ORCID
(National Center for Atmospheric Research Boulder, Colorado, United States)
Owen B. Toon ORCID
(University of Colorado Boulder Boulder, Colorado, United States)
Michael J. Mills ORCID
(National Center for Atmospheric Research Boulder, Colorado, United States)
Francis Vitt ORCID
(National Center for Atmospheric Research Boulder, Colorado, United States)
Lili Xia ORCID
(Rutgers, The State University of New Jersey New Brunswick, New Jersey, United States)
Jonas Jaegermeyr ORCID
(Goddard Institute for Space Studies New York, New York, United States)
Nicole S. Lovenduski ORCID
(University of Colorado Boulder Boulder, Colorado, United States)
Kim J. N. Scherrer ORCID
(Autonomous University of Barcelona Cerdanyola del Vallès, Spain)
Margot Clyne ORCID
(University of Colorado Boulder Boulder, Colorado, United States)
Alan Robock ORCID
(Rutgers, The State University of New Jersey New Brunswick, New Jersey, United States)
Date Acquired
September 5, 2021
Publication Date
September 10, 2021
Publication Information
Publication: Journal of Geophysical Research: Atmospheres
Publisher: Wiley / American Geophysical Union
Volume: 126
Issue: 18
Issue Publication Date: September 27, 2021
ISSN: 2169-897X
e-ISSN: 2169-8996
Subject Category
Meteorology And Climatology
Funding Number(s)
CONTRACT_GRANT: 80NSSC20M0282
Distribution Limits
Public
Copyright
Use by or on behalf of the US Gov. Permitted.
Technical Review
External Peer Committee
Keywords
nuclear war
surface ultraviolet (UV) light
aerosols
photolysis rates
ozone layer
food production
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