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Early Fluid Activity on Ryugu Inferred By Oxygen, Carbon, and 53Mn-53Cr Isotopic Analyses of Carbonates and Magnetite Samples from asteroid Ryugu returned by the Hayabusa2 mission contain evidence of extensive alteration by aqueous fluids and appear related to the CI chondrites. To understand the sources of the fluid and the timing of chemical reactions occurring during the alteration processes, we investigated the oxygen, carbon, and 53Mn-53Cr systematics of carbonate and magnetite in two Ryugu particles. We find that the fluid was initially between 0−20 °C and enriched in 13C, and 17O and 18O, and subsequently evolved towards lighter carbon and oxygen isotopic compositions as alteration proceeded. Carbonate ages show that this fluid-rock interaction took place within the first ~1.8 million years of solar system history, requiring early accretion either in a planetesimal less than ~20 km in diameter or within a larger body which was disrupted and reassembled.
Document ID
20220016690
Acquisition Source
Johnson Space Center
Document Type
Accepted Manuscript (Version with final changes)
Authors
Kaitlyn A McCain ORCID
(Jacobs (United States) Dallas, Texas, United States)
Nozomi Matsuda ORCID
(University of California, Los Angeles Los Angeles, California, United States)
Ming-Chang Liu ORCID
(University of California, Los Angeles Los Angeles, California, United States)
Kevin D McKeegan
(University of California, Los Angeles Los Angeles, California, United States)
Akira Yamaguchi ORCID
(National Institute of Polar Research Tokyo, Japan)
Makoto Kimura ORCID
(National Institute of Polar Research Tokyo, Japan)
Naotaka Tomioka ORCID
(Japan Agency for Marine-Earth Science and Technology Yokosuka, Japan)
Motoo Ito
(Japan Agency for Marine-Earth Science and Technology Yokosuka, Japan)
Naoya Imae
(National Institute of Polar Research Tokyo, Japan)
Masayuki Uesugi ORCID
(Japan Synchrotron Radiation Research Institute Kobe, Japan)
Naoki Shirai ORCID
(Tokyo Metropolitan University Tokyo, Tôkyô, Japan)
Takuji Ohigashi
(Institute for Molecular Science Okazaki, Japan)
Richard C Greenwood
(The Open University Milton Keynes, United Kingdom)
Kentaro Uesugi ORCID
(Japan Synchrotron Radiation Research Institute Kobe, Japan)
Aiko Nakato
(Institute of Space and Astronautical Science Tokyo, Japan)
Kasumi Yogata
(Institute of Space and Astronautical Science Tokyo, Japan)
Hayato Yuzawa
(Institute for Molecular Science Okazaki, Japan)
Yu Kodama
(Marine Works Japan Yokosuka, Kanagawa, Japan)
Kaori Hirahara ORCID
(Osaka University Osaka, Japan)
Ikuya Sakurai ORCID
(Nagoya University Nagoya, Japan)
Ikuo Okada
(Nagoya University Nagoya, Japan)
Yuzuru Karouji
(Institute of Space and Astronautical Science Tokyo, Japan)
Satoru Nakazawa ORCID
(Institute of Space and Astronautical Science Tokyo, Japan)
Tatsuaki Okada ORCID
(Institute of Space and Astronautical Science Tokyo, Japan)
Takanao Saiki ORCID
(Institute of Space and Astronautical Science Tokyo, Japan)
Satoshi Tanaka ORCID
(Institute of Space and Astronautical Science Tokyo, Japan)
Fuyuto Terui
(Kanagawa Institute of Technology Atsugi, Kanagawa, Japan)
Makoto Yoshikawa
(Institute of Space and Astronautical Science Tokyo, Japan)
Akiko Miyazaki ORCID
(Institute of Space and Astronautical Science Tokyo, Japan)
Masahiro Nishimura
(Institute of Space and Astronautical Science Tokyo, Japan)
Toru Yada ORCID
(Institute of Space and Astronautical Science Tokyo, Japan)
Masanao Abe ORCID
(Institute of Space and Astronautical Science Tokyo, Japan)
Tomohiro Usui ORCID
(Institute of Space and Astronautical Science Tokyo, Japan)
Sei-ichiro Watanabe ORCID
(Nagoya University Nagoya, Japan)
Yuichi Tsuda
(Institute of Space and Astronautical Science Tokyo, Japan)
Date Acquired
November 3, 2022
Publication Date
January 12, 2023
Publication Information
Publication: Nature Astronomy
Publisher: Nature Research
Volume: 7
Issue: 3
Issue Publication Date: March 1, 2023
e-ISSN: 2397-3366
Subject Category
Lunar and Planetary Science and Exploration
Funding Number(s)
CONTRACT_GRANT: 80JSC022DA035
Distribution Limits
Public
Copyright
Portions of document may include copyright protected material.
Technical Review
External Peer Committee
Keywords
Astromaterials
Isotope geochemistry
Asteroids, comets and Kuiper belt
Early solar system
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