Statistics of Smoke Sphericity and Optical Properties Using Spaceborne Lidar Measurements

Smoke particles from biomass burning events are typically assumed to be spherical despite previous observations of non-spherical smoke. As such, large uncertainties exist in some physical and optical parameters used in lidar aerosol retrievals, including depolarization and lidar ratio of non-spherical smoke aerosols. In this analysis, using NASA’s Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) data during the biomass burning season over Africa from 2015 to 2017, we studied the frequency and distribution of non-spherical smoke particles to compare with findings of smoke particle non-sphericity from the Cloud-Aerosol Transport System (CATS) lidar. A supplemental smoke aerosol typing algorithm was developed to identify aerosol layers containing non-spherical smoke particles, which might otherwise be misclassified as desert dust, polluted dust, or dusty marine by the CALIOP standard aerosol typing algorithm. Then, the relationships between smoke particle sphericity, lidar ratio, and relative humidity are analyzed for CATS and CALIOP observations over Africa. Approximately 18% of smoke layers observed by CALIOP over Africa are non-spherical (depolarization ratio > 0.075) and agree with spatial distributions of non-spherical smoke found in CATS observations. A dependance of lidar ratio on relative humidity was found for layers of spherical smoke over Africa in both CATS and CALIOP data; however, no such dependance was evident for the depolarization ratio and layer relative humidity. While the supplemental smoke aerosol typing algorithm presented in this analysis was targeted only for specific biomass burning regions during biomass burning seasons and is not meant for global operational use, it presents one potential method for improved backscatter lidar aerosol typing. These results suggest that a dynamic lidar ratio, based on layer-relative humidity for spherical smoke, could be used to reduce uncertainties in smoke aerosol extinction retrievals for future backscatter lidars.