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Tropical Tropospheric Ozone Trends (1998 to 2023): New Perspectives From SHADOZ, IAGOS and OMI/MLS ObservationsTropospheric ozone trends are important indicators of climate forcing and surface pollution, yet relevant satellite observations are too uncertain for assessments. The assessment project TOAR-II has used multi-instrument, ground-based data for global trends over 2000–2022 (Van Malderen et al., 2025a, b). For the tropics, trends are derived from SHADOZ ozonesonde profiles (Thompson et al., 2021, “T21”; Stauffer et al., 2024) or combinations of satellite, SHADOZ and IAGOS aircraft measurements (Gaudel et al., 2024). We extend T21 that covered 1998–2019, analyzing SHADOZ data at five sites with a Multiple Linear Regression (MLR) model for 1998–2023 and reporting trends for two free-tropospheric (FT) segments, the lowermost stratosphere and the total tropospheric column (TrCOsonde). Trends for the Aura period, 2005–2023, are computed from OMI/MLS TrCOsatellite. We find the following: (1) Extending SHADOZ analyses 4 years shows little change from T21; TrCOsonde trends are small (0.5–1 DU/decade) except over SE Asia. (2) Annual trends for TrCOsonde and OMI/MLS TrCOsatellite agree within uncertainties at four of five sites, with the largest differences at Samoa. Sensitivity tests show the following: (a) Adding thousands of FT IAGOS profiles to SHADOZ yields little change in trends; SHADOZ sampling is sufficient. (b) Quantile Regression (QR) and MLR median trends are both near zero, but QR captures extremes (5th percentile, 95th percentile) with changes up to ±1 DU/decade (p< 0.10). (c) Twelve-year analyses for trends lead to uncertainty changes too large for an assessment. (1) This study and Van Malderen et al. (2025a, b) provide the most reliable TOAR-II trends to date: over the past ∼ 25 years, tropical FT ozone changes have been modest, ∼ (−3–+3) %/decade, except over SE Asia.
Document ID
20250011756
Acquisition Source
Goddard Space Flight Center
Document Type
Accepted Manuscript (Version with final changes)
Authors
Anne M Thompson ORCID
(University of Maryland, Baltimore County Baltimore, United States)
Ryan M Stauffer ORCID
(Goddard Space Flight Center Greenbelt, United States)
Debra E Kollonige ORCID
(Science Systems & Applications, Inc. Hampton, VA, USA)
Jerald R Ziemke ORCID
(Morgan State University Baltimore, United States)
Bryan J Johnson ORCID
(NOAA Oceanic and Atmospheric Research Silver Spring, United States)
Gary A Morris ORCID
(NOAA Oceanic and Atmospheric Research Silver Spring, United States)
Patrick Cullis ORCID
(NOAA Oceanic and Atmospheric Research Silver Spring, United States)
Maria Cazorla ORCID
(Instituto de Investigaciones Avícolas Havana, Cuba)
Jorge Andres Diaz
(Universidad de Costa Rica San José, Costa Rica)
Ankie Piters ORCID
(Royal Netherlands Meteorological Institute De Bilt, The Netherlands)
Igor Nedeljkovic ORCID
(Royal Netherlands Meteorological Institute De Bilt, The Netherlands)
Truus Warsodikromo ORCID
(Meteorological Service of Surinam)
Francisco Raimundo Silva ORCID
(Instituto Nacional de Pesquisas Espaciais São José dos Campos, Brazil)
E Thomas Northam
(Science Systems and Applications (United States) Lanham, United States)
Patrick Benjamin ORCID
(United States Space Force Arlington, United States)
Thumeka Mkololo ORCID
(South African Weather Service Pretoria, South Africa)
Tshidi Machinini ORCID
(South African Weather Service Pretoria, South Africa)
Christian Felix ORCID
(Federal Office of Meteorology and Climatology MeteoSwiss Zurich, Switzerland)
Gonzague Romanens ORCID
(Federal Office of Meteorology and Climatology MeteoSwiss Zurich, Switzerland)
Syprose Nyadida ORCID
(Kenya Meteorological Department)
Jerome Brioude ORCID
(Laboratoire de l'Atmosphère et des Cyclones Saint-Denis, Réunion)
Stephanie Evan ORCID
(Laboratoire de l'Atmosphère et des Cyclones Saint-Denis, Réunion)
Jean-Marc Metzger ORCID
(Observatoire des Sciences de l'Univers de la Réunion Saint-Denis, Réunion)
Ambun Dindang ORCID
(Malaysian Meteorological Department)
Yuzaimi B Mahat ORCID
(Malaysian Meteorological Department)
Mohan Kumar Summathuria ORCID
(Malaysian Meteorological Department)
Norazura Binti Zakaria ORCID
(Malaysian Meteorological Department)
Ninong Komala ORCID
(National Research and Innovation Agency Jakarta, Indonesia)
Shin-Ya Ogino ORCID
(Japan Agency for Marine-Earth Science and Technology Yokosuka, Japan)
Nguyen Thi Quyen ORCID
(Aero-Meteorological Observatory)
Francis S Mani ORCID
(University of the South Pacific Suva, Fiji)
Miriama Vuiyasawa ORCID
(University of the South Pacific Suva, Fiji)
David Nardini ORCID
(University of Hawaiʻi at Mānoa Honolulu, United States)
Matthew Martinsen ORCID
(University of Colorado Boulder Boulder, United States)
Darryl T Kuniyuki ORCID
(National Oceanic and Atmospheric Administration Washington, United States)
Katrin Muller
(Alfred - Wegener - Institut)
Pawel Wolff ORCID
(Université Toulouse III - Paul Sabatier Toulouse, France)
Bastien Sauvage ORCID
(Laboratoire d'Aérologie Toulouse, France)
Date Acquired
December 30, 2025
Publication Date
December 19, 2025
Publication Information
Publication: Atmospheric Chemistry and Physics
Publisher: Copernicus.org (Germany)
Volume: 25
Issue: 24
Issue Publication Date: December 19, 2025
ISSN: 1680-7316
e-ISSN: 1680-7324
Subject Category
Meteorology and Climatology
Funding Number(s)
WBS: 281945.02.80.01.06
WBS: 437949.02.04.01.10
WBS: 509496.02.04.01.10
Distribution Limits
Public
Copyright
Portions of document may include copyright protected material.
Technical Review
NASA Peer Committee
Keywords
tropospheric ozone trends
SHADOZ
tropical ozone
ozone
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