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Increase and seasonal cycles of nitrous oxide in the earth's atmosphereIt is determined that nitrous oxide (N2O) is increasing at about 0.9 ppb/yr in the northern hemisphere and at about 0.7 ppb/yr in the southern hemisphere, based on about 9000 ground-level measurements at Cape Meares, Oregon (45 deg N), and Cape Grim, Tasmania (42 deg S), spanning a three-year period. It is also shown that the N2O concentrations vary with season in the northern hemisphere, where the concentrations are 0.8 ppbv higher during April, May, and June compared to the rest of the year, and in the southern hemisphere where the concentrations are about 0.5 ppbv lower during March, April, and May compared to the rest of the year. An explanation of this increase as a sizeable anthropogenically-controlled land-based source is presented, based on an examination of the existing estimates of natural and anthropogenic sources of N2O. Mass-balance calculations are also presented which suggest that a natural land-based source, peaking in spring, would explain the main features of the observed seasonal cycle. A growth model is employed to extrapolate the observed increase of N2O into the future and the results are compared with exponential extrapolations.
Document ID
19830059426
Acquisition Source
Legacy CDMS
Document Type
Reprint (Version printed in journal)
Authors
Khalil, M. A. K.
(Oregon Graduate Center for Study and Research Beaverton, OR, United States)
Rasmussen, R. A.
(Oregon Graduate Center Beaverton, OR, United States)
Date Acquired
August 11, 2013
Publication Date
July 1, 1983
Publication Information
Publication: Tellus, Series B - Chemical and Physical Meteorology
Volume: 35B
ISSN: 0280-6509
Subject Category
Geophysics
Accession Number
83A40644
Funding Number(s)
CONTRACT_GRANT: NSG-7457
Distribution Limits
Public
Copyright
Other

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