Ozone and water vapor monitoring using a ground-based lidar system

Measurements of atmospheric ozone and water vapor profiles obtained using a differential absorption lidar (DIAL) technique at Haute Provence Observatory are reported. The DIAL technique is based on the comparison of differences in attenuation in backscattered signals at wavelengths centered on strong absorptions or absorption lines of the species in question, and wavelengths corresponding to weaker or no absorption. The system in use is based on three lasers - a Nd:YAG Q-switched laser frequency doubled to emit at 532 nm, and two tunable narrowline dye lasers used to convert this emission into the IR or UV spectral regions. Ozone concentration profiles have been recorded up to a height of 30 km, and reveal large day-to-day variations in number density which were correlated with a decrease in tropopause height. Measurements of water vapor concentrations show a variability of the mixing ratio at heights up to 2.5 km representative of dynamic processes, and a variability above 2.5 km that is within the measurement error. Day-to-day variations in tropospheric mixing ratio were also observed.