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Concentrations and uncertainties of stratospheric trace species inferred from limb infrared monitor of the stratosphere data. I - Methodology and application to OH and HO2. II - Monthly averaged OH, HO2, H2O2, and HO2NO2Difficulties arise in connection with the verification of multidimensional chemical models of the stratosphere. The present study shows that LIMS data, together with a photochemical equilibrium model, may be used to infer concentrations of a variety of zonally averaged trace Ox, OHx, and NOx species over much of the stratosphere. In the lower stratosphere, where the photochemical equilibrium assumption for HOx species breaks down, inferred concentrations should still be accurate to about a factor of 2 for OH and 2.5 for HO2. The algebraic nature of the considered model makes it possible to see easily to the first order the effect of variation of any model input parameter or its uncertainty on the inferred concontration of the HOx species and their uncertainties.
Document ID
19860042257
Document Type
Reprint (Version printed in journal)
Authors
Kaye, J. A. (NASA Goddard Space Flight Center Greenbelt, MD, United States)
Jackman, C. H. (NASA Goddard Space Flight Center Greenbelt, MD, United States)
Date Acquired
August 12, 2013
Publication Date
January 20, 1986
Publication Information
Publication: Journal of Geophysical Research
Volume: 91
ISSN: 0148-0227
Subject Category
GEOPHYSICS
Distribution Limits
Public
Copyright
Other