Laminar Soot Processes

Soot formation within hydrocarbon-fueled flames is an important unresolved problem of combustion science for several reasons: soot emissions are responsible for more deaths than any other combustion pollutant, thermal loads due to continuum radiation from soot limit the durability of combustors, thermal radiation from soot is mainly responsible for the growth and spread of unwanted fires, carbon monoxide associated with soot emissions is responsible for most fire deaths, and limited understanding of soot processes is a major impediment to the development of computational combustion. Thus, soot processes within laminar nonpremixed (diffusion) flames are being studied, emphasizing space-based experiments at microgravity. The study is limited to laminar flames due to their experimental and computational tractability, noting the relevance of these results to practical flames through laminar flamelet concepts. The microgravity environment is emphasized because buoyancy affects soot processes in laminar diffusion flames whereas effects of buoyancy are small for most practical flames. Results discussed here were obtained from experiments carried out on two flights of the Space Shuttle Columbia. After a brief discussion of experimental methods, results found thus far are described, including soot concentration measurements, laminar flame shapes, laminar smoke points and flame structure. The present discussion is brief.