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New Particle Formation and Growth to Climate‐Relevant Aerosols at a Background Remote Site in the Western HimalayaNew particle formation (NPF) can influence the Earth's radiative budget when the newly formed particles grow to climate‐relevant sizes. Here, we present analysis of 21 months of continuous aerosol size distribution measurements at a background remote site in the western Himalaya and provide observational evidence that newly formed particles grow to cloud condensation nuclei (CCN)‐active sizes (i.e., >20–100 nm in diameter). Out of total 55 NPF events, 38 (66%) events occurred in the pre‐monsoon season (March–May). NPF events were classified into those with and without pollution influence as polluted and cleaner, respectively, using black carbon data. The analysis of air mass age, based on the ratio of number concentration of Aitken to accumulation mode aerosols, indicated that NPF occurred in the relatively cleaner air masses reaching to the site. The median formation rate of 10 nm particles and particle growth rates for cleaner events were three‐fold and two‐fold, respectively, higher than polluted events. We present the first estimates of the survival probability of newly formed particles to 50 and 100 nm size, which was not attempted in an Indian environment previously. The survival probability to 50 nm particles ranged from 44% to 98%, with a mean and standard deviation of 82 ± 18%. On average, ∼60% of the particles surviving to 50 nm survived to 100 nm, making the overall survival probability of 100 nm to 53 ± 31%. This indicates that the probability of nucleated particles growing to CCN‐active sizes under a large source of condensing vapor (transported from nearby lower‐altitude regions) and low pre‐existing particle concentrations (background mountain site) is high compared to the previous studies. These findings highlight the importance of the efficiency of nucleation events for producing CCN, which is a critical basis of aerosol indirect effects.
Document ID
20210014184
Acquisition Source
Goddard Space Flight Center
Document Type
Accepted Manuscript (Version with final changes)
Authors
Mathew Sebastian
(University of Hyderabad Hyderabad, India)
Vijay P. Kanawade ORCID
(University of Hyderabad Hyderabad, India)
Vijay K. Soni
(Ministry of Earth Sciences New Delhi, India)
Eija Asmi
(Finnish Meteorological Institute Helsinki, Finland)
Daniel. M. Westervelt ORCID
(Lamont-Doherty Earth Observatory Sparkill, New York, United States)
Ville Vakkari
(Finnish Meteorological Institute Helsinki, Finland)
Antti-Pekka Hyvärinen
(Finnish Meteorological Institute Helsinki, Finland)
Jeffrey R. Pierce ORCID
(Colorado State University Fort Collins, Colorado, United States)
Rakesh Hooda ORCID
(Finnish Meteorological Institute Helsinki, Finland)
Date Acquired
April 21, 2021
Publication Date
April 1, 2021
Publication Information
Publication: Journal of Geophysical Research: Atmospheres
Publisher: American Geophysical Union / Wiley
Volume: 126
Issue: 7
Issue Publication Date: April 16, 2021
ISSN: 2169-897X
e-ISSN: 2169-8996
Subject Category
Meteorology And Climatology
Funding Number(s)
CONTRACT_GRANT: 80NSSC17M0057
CONTRACT_GRANT: ECR/2016/001333
CONTRACT_GRANT: DE-SC0019000
Distribution Limits
Public
Copyright
Use by or on behalf of the US Gov. Permitted.
Technical Review
External Peer Committee
Keywords
cloud condensation nuclei
new particle formation
particle growth
the Himalaya
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